Learn the tune Cajun Hot Shoe. One of the single most strenuous tunes for Cajun accordion, thank I've ever played, anyway... The amount of back and forth you have to do really makes you appreciate songs that don't require constant push pull
No pain, no gain I'm finally off a lazy plateau thanks to this tune.
Re: something that can make your playing better....
Another excellent tune to learn is the "Domino Two Step" by Nathan Abshire. This tune will build speed and dexterity in your fingers. I purchased it from iTunes and learned it with the Amazing Slowdowner. It took a while but it was well worth the effort.